Harvest Moon - Neil Young
(This song got me interested in N. Young, I first heard it in the film Away from Her (2006), and Harvest Moon is still my favourite Neil Young album.)
Neil Young - Harvest Moon
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The Promise - When in Rome
(The "nerd" movie Napoleon Dynamite uses this track in the end credits. IMO not the best film, the dance scene in the movie is a classic, though. ( ;
Gin Soaked Boy - The Divine Comedy
(This song is amazing, he even includes 'The Catcher in the Rye' in the lyrics!)